Distribution of localized states from fine analysis of electron spin resonance spectra of organic semiconductors: Physical meaning and methodology

We develop an analytical method for the processing of electron spin resonance (ESR) spectra. The goal is to obtain the distributions of trapped carriers over both their degree of localization and their binding energy in semiconductor crystals or films composed of regularly aligned organic molecules [Phys. Rev. Lett. v. 104, 056602 (2010)]. Our method has two steps. We first carry out a fine analysis of the shape of the ESR spectra due to the trapped carriers; this reveals the distribution of the trap density of the states over the degree of localization. This analysis is based on the reasonable assumption that the linewidth of the trapped carriers is predetermined by their degree of localization because of the hyperfine mechanism. We then transform the distribution over the degree of localization into a distribution over the binding energies. The transformation uses the relationships between the binding energies and the localization parameters of the trapped carriers. The particular relation for the system under study is obtained by the Holstein model for trapped polarons using a diagrammatic Monte Carlo analysis. We illustrate the application of the method to pentacene organic thin-film transistors.Comment: 14 pages, 11 figure

Stability analysis of some integrable Euler equations for SO(n)

A family of special cases of the integrable Euler equations on $so(n)$ introduced by Manakov in 1976 is considered. The equilibrium points are found and their stability is studied. Heteroclinic orbits are constructed that connect unstable equilibria and are given by the orbits of certain 1-parameter subgroups of SO(n). The results are complete in the case $n=4$ and incomplete for $n>4$.Comment: 15 pages, LaTeX, minor stylistic changes in v

Polaron in t-J model

We present numeric results for ground state and angle resolved photoemission spectra (ARPES) for single hole in t-J model coupled to optical phonons. The systematic-error free diagrammatic Monte Carlo is employed where the Feynman graphs for the Matsubara Green function in imaginary time are summed up completely with respect to phonons variables, while magnetic variables are subjected to non-crossing approximation. We obtain that at electron-phonon coupling constants relevant for high Tc cuprates the polaron undergoes self-trapping crossover to strong coupling limit and theoretical ARPES demonstrate features observed in experiment: a broad peak in the bottom of the spectra has momentum dependence which coincides with that of hole in pure t-J model.Comment: 4 pages, 4 figure